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Vibrations de valence C-H des alcanes et halogénures de t-butyle

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Ion Spectroscopy Reveals Structural Difference for Proteins Microhydrated by Retention and Condensation of Water

Oleg Boyarkine, Andrei Zviagin

Protein ubiquitin in its +7 charge state microhydrated by 5 and 10 water molecules has been interrogated in the gas phase by cold ion UV/IR spectroscopy. The complexes were formed either by condensing water onto the unfolded bare proteins in a temperature- ...

Amer Chemical Soc2024

Vibrational NDT with Under-sampled Data through Physics-informed Neural Networks

Olga Fink

The vibrational response of solid materials and structural components is substantially governed by their mechanical and geometrical properties. Low-frequency vibrations and modal frequencies are sensitive to global geometrical deviations, while high-freque ...

2023

Antenna-coupled infrared nanospectroscopy of intramolecular vibrational interaction

Hatice Altug, Aurélian Michel John-Herpin

Many photonic and electronic molecular properties, as well as chemical and biochemical reactivities are controlled by fast intramolecular vibrational energy redistribution (IVR). This fundamental ultrafast process limits coherence time in applications from ...

National Academy of Sciences2023

Imaging and controlling coherent phonon wave packets in single graphene nanoribbons

Klaus Kern

The motion of atoms is at the heart of any chemical or structural transformation in molecules and materials. Upon activation of this motion by an external source, several (usually many) vibrational modes can be coherently coupled, thus facilitating the che ...

Nature Portfolio2023

Single molecule fluorescence and phosphorescence studies using a scanning tunneling microscope

Abhishek Grewal

This thesis investigates novel single-molecule luminescence phenomena at their inherent, sub-molecular length scale. The microscopic understanding of luminescence processes will be crucial for the continued improvement of organic optoelectronic and semicon ...

EPFL2022

State-to-state surface scattering of methane studied by bolometric infrared laser tagging detection

Bo-Jung Chen

State-to-state molecule/surface scattering experiments prepare the incident molecules in a specific quantum state and measure the quantum state distribution of the scattered molecules. The comparison of state resolved experiments with theory can serve as s ...

EPFL2022

Structure-property relationships and mixed conductivity in layered hybrid perovskites based on phenyl-derived spacers

Algirdas Ducinskas

Hybrid halide perovskites are currently one of the most studied semiconductors. However, due to poor intrinsic and extrinsic stability, further developments to commercialize devices based on hybrid halide perovskites are limited. Many different strategies ...

EPFL2022

Optically reconfigurable quasi-phase-matching in silicon nitride microresonators

Camille Sophie Brès, Jianqi Hu, Edgars Nitiss, Anton Stroganov

Quasi-phase-matching has long been a widely used approach in nonlinear photonics, enabling efficient parametric frequency conversions such as second-harmonic generation. However, in silicon photonics the task remains challenging, as materials best suited f ...

Nature Publishing Group2022

Seeded Multimode Quasi-Phase-Matching in All-Optically Poled Silicon Nitride Waveguides

Camille Sophie Brès, Edgars Nitiss, Ozan Yakar

We demonstrate seeding-enabled all-optical poling of silicon nitride waveguides as short as 5 mm, and account for quasi-phase-matching (QPM) inside the waveguide between the fundamental mode of pump and higher order second-harmonic modes. ...

OSA2021

Broadband visible two-dimensional spectroscopy of molecular dyes

Majed Chergui, Andre Al Haddad, Rebecca Ann Ingle, Lars-Hendrik Mewes

Two-dimensional Fourier transform spectroscopy is a promising technique to study ultrafast molecular dynamics. Similar to transient absorption spectroscopy, a more complete picture of the dynamics requires broadband laser pulses to observe transient change ...

AMER INST PHYSICS2021

Studies of cold chemistry in crossed and merged neutral beams

Silvia Tanteri

In this thesis we present the design of two setups to study low-energy collisions between neutral species: an electron velocity map imaging for chemi-ionisation reactions and a merged electrostatic guide for polar molecules scattering. In the past few yea ...

EPFL2021

Vibrational Sum Frequency Scattering in Absorptive Media: A Theoretical Case Study of Nano-objects in Water

Sylvie Roke, Saranya Pullanchery Sankara Narayanan, Sergey Kulik

The structures of interfaces of nano- and microscale objects in an aqueous solution are important for a wide variety of physical, chemical, and biological processes. Vibrational sum frequency (SF) scattering has emerged as a useful and unique probe of the ...

AMER CHEMICAL SOC2020

Phonon-Ion Interactions: Designing Ion Mobility Based on Lattice Dynamics

Sokseiha Muy

This review is focused on the influence of lattice dynamics on the ionic mobility in superionic conductors in particular solid-state Li-ion conductors. After a succinct review of the static view of ionic conduction, the role of polarizability as the underl ...

WILEY-V C H VERLAG GMBH2020

Raman spectroscopy and lattice dynamics calculations of tetragonally-structured single crystal zinc phosphide (Zn3P2) nanowires

Anna Fontcuberta i Morral, Jean-Baptiste Leran, Mahdi Zamani, Simon Robert Escobar Steinvall, Elias Zsolt Stutz, Rajrupa Paul, Mirjana Dimitrievska

Earth-abundant and low-cost semiconductors, such as zinc phosphide (Zn3P2), are promising candidates for the next generation photovoltaic applications. However, synthesis on commercially available substrates, which favors the formation of defects, and cont ...

2020

High-Q surface electromagnetic wave resonance excitation in magnetophotonic crystals for supersensitive detection of weak light absorption in the near-infrared

Serguei Sekatski

The mid-infrared spectrum can be recorded from almost any material, making mid-infrared spectroscopy an extremely important and widely used sample characterization and analysis technique. However, sensitive photoconductive detectors operate primarily in th ...

OPTICAL SOC AMER2020

Radiative cooling of carbon cluster anions C-2n+1(-) (n=3-5)

Eduardo Carrascosa Casado

Radiative cooling of carbon cluster anions C(2n+1)(-)C2n+1- (n = 3-5) is investigated using the cryogenic electrostatic ion storage ring DESIREE. Two different strategies are applied to infer infrared emission on slow (milliseconds to seconds) and ultraslo ...

SPRINGER2020

Physics of optically driven nanojunctions

Philippe Andreas Rölli

Recent years have seen spectacular developments in the domain of nano-optics. Alongside the well-known techniques of super-resolution microscopy progress in nanofabrication has enabled important improvements in the fields of optical imaging and spectros ...

EPFL2020

Unimolecular fragmentation and radiative cooling of isolated PAH ions: A quantitative study

Eduardo Carrascosa Casado

Time-resolved spontaneous and laser-induced unimolecular fragmentation of perylene cations (C20H12+) has been measured on timescales up to 2 s in a cryogenic electrostatic ion beam storage ring. We elaborate a quantitative model, which includes fragmentati ...

AMER INST PHYSICS2020

Doubly resonant second-harmonic generation of a vortex beam from a bound state in the continuum

Nicolas Grandjean, Romuald Houdré, Jean-François Carlin, Matteo Galli, Momchil Minkov, Marco Clementi, Jun Wang

Second-harmonic generation in nonlinear materials can be greatly enhanced by realizing doubly resonant cavities with high quality factors. However, fulfilling such doubly resonant condition in photonic crystal (PhC) slab cavities is a long-standing challen ...

2020

Preparation and Decay of a Single Quantum of Vibration at Ambient Conditions

Christophe Marcel Georges Galland, Vivishek Sudhir, Mitchell David Anderson, Santiago Tarrago Velez, Kilian Robert Seibold

A single quantum of excitation of a mechanical oscillator is a textbook example of the principles of quantum physics. But mechanical oscillators, despite their pervasive presence in nature and modem technology, do not genetically exist in an excited Fock s ...

American Physical Society2019