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Plasmonic nanostructures have shown great promise in solar thermal applications. Here we report highly efficient solar vapor generation using hollow-mesoporous plasmonic nanoshells, where the steam production is significantly enhanced by the extended active surface and the nearly neutral buoyancy. An energy-to-vapor conversion efficiency of 69% was measured under 10x solar irradiance. We also show clear evidence of direct vapor nucleation from the plasmonic structure without bulk heating.
Fernando Porté Agel, Mohammad Jamshidmofid
Michael Graetzel, Shaik Mohammed Zakeeruddin, Felix Thomas Eickemeyer