Temporal and spectral shaping of broadband terahertz pulses in a photoexcited semiconductor

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Integrated photonic circuits for terahertz applications

This talk will discuss recent advances in the nascent field of integrated photonic circuits for terahertz applications. This field explores photonic circuit technology to create miniaturized terahertz emitters and detectors by non-linear optical processes ...

IEEE2022

Spatio-Temporal Dynamics of Free and Bound Carriers in Photovoltaic Materials

Jacques-Edouard Moser, George Cameron Fish

Photoinduced charge separation into free carriers and subsequent charge transfer are key processes that govern the efficiencies of third generation solar cell technologies based on donor-acceptor heterojunctions. As these processes typically occur on picos ...

2022

Ultrafast carrier and quasiparticle dynamics in strongly confined perovskite nanoplatelets

Etienne Christophe Socie

Over the past decade, lead halide perovskites (LHPs) have received considerable attention thanks to their impressive optoelectronic properties. Today, LHP-based devices are one of the most efficient single-junction solar cells, with power-conversion effici ...

EPFL2022

Ultrashort Pulse Excited Tip-Enhanced Raman Spectroscopy in Molecules

Klaus Kern, Yang Luo

Vibrational fingerprints of molecules and lowdimension materials can be traced with subnanometer resolution by performing Tip-enhanced Raman spectroscopy (TERS) in a localization of light in the plasmonic nanocavity of the STM enables high spatial resoluti ...

AMER CHEMICAL SOC2022

Highly efficient THz four-wave mixing in doped silicon

Gabriel Aeppli

Third-order non-linearities are important because they allow control over light pulses in ubiquitous high-quality centro-symmetric materials like silicon and silica. Degenerate four-wave mixing provides a direct measure of the third-order non-linear sheet ...

SPRINGERNATURE2021

Coherent terahertz-to-microwave link using electro-optic-modulated Turing rolls

Tobias Kippenberg, Miles Henry Anderson, Arslan Sajid Raja, Wenle Weng, Jijun He, Anat Siddharth

Arising from modulation instability, Turing rolls in optical Kerr microresonators have been used in the generation of optical frequency combs and the synthesis of microwave and terahertz frequencies. In this work, by applying electro-optic modulation on te ...

AMER PHYSICAL SOC2021

Methylammonium Triiodide for Defect Engineering of High-Efficiency Perovskite Solar Cells

Michael Graetzel, Jacques-Edouard Moser, Shaik Mohammed Zakeeruddin, Mounir Driss Mensi, Ursula Röthlisberger, Ulf Anders Hagfeldt, Thomas Paul Baumeler, Linfeng Pan, Paramvir Ahlawat, Claudia Esther Avalos, Essa Awadh R Alharbi, Pascal Alexander Schouwink, George Cameron Fish, Mathias Dankl, Bowen Yang, Felix Thomas Eickemeyer, Viktor Skorjanc, Anurag Krishna, Olivier Ouellette, Elsa John, Lukas Pfeifer

The defects present in metal halide perovskite are deleterious to both the performance and stability of photovoltaic devices. Consequently, there is an intense focus on developing defect mitigation strategies. Herein we report a facile strategy that employ ...

2021

Resonant Band-Edge Emissive States in Strongly Confined CsPbBr3 Perovskite Nanoplatelets

Jacques-Edouard Moser, Etienne Christophe Socie, Aaron Tomas Terpstra, Brener Rodrigo De Carvalho Vale

Strongly confined, fully inorganic cesium lead halide perovskite nanocrystals are of great promise for light-emitting devices in the blue spectral range owing to their high photoluminescence quantum yields. A combination of broadband fluorescence up-conver ...

2021

Ultrafast Photon-Induced Tunneling Microscopy

Klaus Kern, Yang Luo

Unification of the techniques of ultrafast science and scanning tunneling microscopy (STM) has the potential of tracking electronic motion in molecules simultaneously in real space and real time. Laser pulses can couple to an STM junction either in the wea ...

AMER CHEMICAL SOC2021

Ultra-broadband time-resolved THz spectroscopy of perovskites and nanomaterials

Andrés Burgos Caminal

The fundamental study of charge carrier dynamics has been shown to be of great interest for optoelectronics, paving the way forward for future developments. Often, some of the key processes that determine the photophysics of a material occur on very short ...

EPFL2020

Molecular Platform for Frequency Upconversion at the Single-Photon Level

Christophe Marcel Georges Galland, Tobias Kippenberg, Philippe Andreas Rölli

Direct detection of single photons at wavelengths beyond 2 mu m under ambient conditions remains an outstanding technological challenge. One promising approach is frequency upconversion into the visible (VIS) or near-infrared (NIR) domain, where single-pho ...

American Physical Society2020

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