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Inelastic neutron scattering, susceptibility, and high-field magnetization identify LiCuVO4 as a nearest-neighbour ferromagnetic, next-nearest-neighbour frustrated, quasi-one-dimensional helimagnet, which is largely influenced by quantum fluctuations. Complementary band structure calculations provide a microscopic model with the correct sign and magnitude of the major exchange integrals.
Christian Wäckerlin, Quy Hien Le, Diego Radillo Ochoa, Céline Hensky